Designer photonic dynamics by using non-uniform electron temperature distribution for on-demand all-optical switching times

Research output: Contribution to journalArticlepeer-review

36 Citations (Scopus)
127 Downloads (Pure)

Abstract

While free electrons in metals respond to ultrafast excitation with refractive index changes on femtosecond time scales, typical relaxation mechanisms occur over several picoseconds, governed by electron-phonon energy exchange rates. Here, we propose tailoring these intrinsic rates by engineering a non-uniform electron temperature distribution through nanostructuring, thus, introducing an additional electron temperature relaxation channel. We experimentally demonstrate a sub-300 fs switching time due to the wavelength dependence of the induced hot electron distribution in the nanostructure. The speed of switching is determined by the rate of redistribution of the inhomogeneous electron temperature and not just the rate of heat exchange between electrons and phonons. This effect depends on both the spatial overlap between control and signal fields in the metamaterial and hot-electron diffusion effects. Thus, switching rates can be controlled in nanostructured systems by geometrical parameters and selected wavelengths, which determine the control and signal mode distributions.
Original languageEnglish
Article number2967
JournalNature Communications
Volume10
Issue number1
DOIs
Publication statusPublished - 1 Dec 2019

Fingerprint

Dive into the research topics of 'Designer photonic dynamics by using non-uniform electron temperature distribution for on-demand all-optical switching times'. Together they form a unique fingerprint.

Cite this