High Harmonic Generation in Two-Dimensional Mott Insulators

Chris Orthodoxou, Amelle Zair, George H. Booth*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

138 Downloads (Pure)

Abstract

With a combination of numerical methods, including quantum Monte Carlo, exact diagonalization, and a simplified dynamical mean-field model, we consider the attosecond charge dynamics of electrons induced by strong-field laser pulses in two-dimensional Mott insulators.
The necessity to go beyond single-particle approaches in these strongly correlated systems has made the simulation of two-dimensional extended materials challenging, and we contrast their resulting high-harmonic emission with more widely studied one-dimensional analogues. As well as considering the photo-induced breakdown of the Mott insulating state and magnetic order, we also resolve the time and ultra-high frequency domains of emission, which are used to characterize both the photo-transition, and the sub-cycle structure of the electron dynamics. This extends simulation capabilities and understanding of the photo-melting of these Mott insulators in two-dimensions, at the frontier of attosecond non-equilibrium science of correlated materials.
Original languageEnglish
Number of pages10
JournalNPJ Quantum Materials
Publication statusAccepted/In press - 13 Jul 2021

Fingerprint

Dive into the research topics of 'High Harmonic Generation in Two-Dimensional Mott Insulators'. Together they form a unique fingerprint.

Cite this